Exciton Dynamics in Lead Halide Perovskite Nanocrystals

Recombination, Dephasing and Diffusion
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Less than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission. 
 In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as the active layer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before.


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ReiheSpringer Theses
ISBN 9783030709426
Sprache Englisch
Ausgabe 1st ed. 2021
Erscheinungsdatum 20.05.2022
Umfang 152 Seiten
Genre Technik/Sonstiges
Format Taschenbuch
Verlag Springer International Publishing